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俞磊教授在Chemical Communications上发表论文
发布日期:2017-12-12浏览次数:字号:[ ]

A divergent [5+2] cascade approach to bicyclo[3.2.1]octanes: facile synthesis of ent-kaurene and cedrene-type skeletons

Chi Hea, Zengbing Bai,b, Jialei Hu,a, Bingnan Wanga, Hujun Xie*,c, Lei Yu*,b and Hanfeng Ding*,a

a Department of Chemistry, Zhejiang University
b School of Chemistry and Chemical Engineering, Yangzhou University,
c Department of Applied Chemistry, Zhejiang Gongshang University,
Electronic supplementary information (ESI) available. CCDC 1543770 (5j), 1557744 (5l), 1543771 (6a0) and 1543772 (15b). For ESI and crystallographic data in CIF or other electronic format see DOI: 10.1039/c7cc04292b
Z. B. and J. H. contributed equally to this work

Abstract: A solvent-dependent oxidative dearomatization-induced divergent [5+2] cascade approach to bicyclo[3.2.1]octanes was described. This novel protocol enables a facile synthesis of a series of diversely functionalized ent-kaurene and cedrene-type skeletons in good yields and excellent diastereoselectivities.

Chemical Communications, 2017, 53, 8435--8438.  IF=6.319

文章链接:http://pubs.rsc.org/en/content/articlelanding/2017/cc/c7cc04292b#!divAbstract




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